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Continuous preparation of carbon-nanotube-supported platinum catalysts in a flow reactor directly heated by electric current

机译:在电流直接加热的流动反应器中连续制备碳纳米管负载的铂催化剂

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摘要

In this contribution we present for the first time a continuous process for the production of highly active Pt catalysts supported by carbon nanotubes by use of an electrically heated tubular reactor. The synthesized catalysts show a high degree of dispersion and narrow distributions of cluster sizes. In comparison to catalysts synthesized by the conventional oil-bath method a significantly higher electrocatalytic activity was reached, which can be attributed to the higher metal loading and smaller and more uniformly distributed Pt particles on the carbon support. Our approach introduces a simple, time-saving and cost-efficient method for fuel cell catalyst preparation in a flow reactor which could be used at a large scale.
机译:在这一贡献中,我们首次提出了使用电加热管式反应器生产由碳纳米管负载的高活性Pt催化剂的连续方法。合成的催化剂显示出高度分散性和簇尺寸的窄分布。与通过常规油浴方法合成的催化剂相比,达到了明显更高的电催化活性,这可以归因于更高的金属负载量和碳载体上更小且更均匀分布的Pt颗粒。我们的方法引入了一种简单,省时且经济高效的方法,用于在流动反应器中制备燃料电池催化剂,可以大规模使用。

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